Sixty-six is a triangular number, the sum of the integers one through eleven, and reduces to twelve and then three. Its most widely recognised meaning is the count of books in the Protestant Bible, thirty-nine in the Old Testament and twenty-seven in the New, so that sixty-six is shorthand for the whole of scripture as reckoned in the Reformed tradition, against the seventy-three of the Catholic canon, which includes the deuterocanonical books. The number owes this significance entirely to the particular canon settled at the Reformation rather than to any symbolic property.
In chemistry, sixty-six is the atomic number of dysprosium, named from the Greek dysprositos, hard to get at, a name its discoverer Paul-Emile Lecoq de Boisbaudran chose in 1886 after more than thirty attempts to separate it out from holmium oxide.
Sixty-six factors as 2 x 3 x 11 and carries 8 divisors in all. Summing its proper divisors gives 78, more than the number itself, which makes it an abundant number in the classical sense the Pythagoreans used to sort integers into deficient, perfect and abundant classes.
The whole apparatus of digit-reduction numerology is a twentieth-century invention rather than an inheritance from antiquity. Mrs. L. Dow Balliett published the first systematic version, The Philosophy of Numbers, in 1908, fixing the letter-to-number chart still used today and ruling that eleven and twenty-two must stand as master numbers rather than reduce further; her colleague, the physician Julia Seton, is credited with coining the word numerology itself around 1912.